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5. lM on the activity of atisvarious activitiespotential of the ions form insoluble Ag salts and there no diffusion representsexperimental the theoretical prediction across membrane. solid lineobserved and thethedotted line theThecommonly dependence. C, c i-, - log ac1 = I - log ac1 = 2 - log ac1 = 3 4 5 6 7 8 9 10 The theory ofmembrane potentials in ISEs 50 reaction in this kind of ISE is discussed theoretically by Hulanicki and Lewenstam [29, 30, 31]. Dissolution ofmembranes with complex formation [ l , 7, 27, 38, 39, 44, 45, 49].

3. 3) = If the ISE membrane is in contact on both sides with solutions of the same ion whose activity is to be determined in the analyte ( determinand J), and neither the analysed nor the internal ISE solution contains another ion that would affect the membrane potential (interferent K), then the membrane potential is AM = (RT/zF) ln [a1( l)/a1(2)], (3. 4) where z is the charge number of ion J and a1( 1) and a1(2) are its activities in solutions 1 and 2. Equation (3. 4) is identical with the Nernst equation for the The theory ofmembrane potentials in ISEs 28 potential of a concentration cell without transfer.

Macinnes and Y. L. Yeh, J. Am. Chem. Soc. 43, 2563 ( 192 1). 23 0. R. Melroy and R. P. Buck, J. Electroanal. Chem. 136, 19 (1 982). 24 W. E. Morf, Anal Chem. 49, 8 10 ( 1 977). 25 W. E. Morf, The Principles ofJon-Selective Electrodes and ofMembrane Transport, Akademiai Kiad6, Budapest ( 1981). 26 W. Nernst, Z. Physik. Chem. 2, 613 ( 1 889). 27 W. Nernst, Z. Physik. Chem. 4 , 129 ( 1 889). 28 W. Nernst and E. H. Riesenfeld, Ann. Phys. 8, 600 ( 1902). 29 A. J. Parker, Electrochim. Acta, 2 1 , 6 7 1 ( 1 976).

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5H superHeavy Hydrogen by A.V. BELOZYOROV,


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